Photocatalytic water splitting into H2 and O2 over various tantalate photocatalysts

書誌事項

公開日
2003-02
権利情報
  • https://www.elsevier.com/tdm/userlicense/1.0/
  • https://www.elsevier.com/legal/tdmrep-license
DOI
  • 10.1016/s0920-5861(02)00355-3
公開者
Elsevier BV

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説明

Photocatalytic water splitting into H 2 and O 2 over various tantalates was reviewed and factors affecting photocatalytic activities of tantalates were discussed from a viewpoint of the crystal structure and the energy structure. Many tantalates, K 3 Ta 3 Si 2 O 13 , alkali and alkaline earth tantalates, were highly active photocatalysts for water splitting. The high activities were mainly due to the high conduction band level consisting of Ta5d orbitals. NiO-loaded NaTaO 3 with the distorted perovskite structure showed the highest activity among tantalates. Moreover, the activity of the NiO/NaTaO 3 photocatalyst was remarkably improved by doping of lanthanoids. The apparent quantum yield of NiO/NaTaO 3 doped with lanthanum was ca. 50% at 270 nm.

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