Highly Stretchable, Elastic, and Ionic Conductive Hydrogel for Artificial Soft Electronics

  • Yang Zhou
    School of Materials Science and Engineering Nanyang Technological University 50 Nanyang Avenue Singapore 639798 Singapore
  • Changjin Wan
    School of Materials Science and Engineering Nanyang Technological University 50 Nanyang Avenue Singapore 639798 Singapore
  • Yongsheng Yang
    School of Chemistry and Engineering Wuhan Textile University 1 Textile Road Wuhan 430073 China
  • Hui Yang
    School of Materials Science and Engineering Nanyang Technological University 50 Nanyang Avenue Singapore 639798 Singapore
  • Shancheng Wang
    School of Materials Science and Engineering Nanyang Technological University 50 Nanyang Avenue Singapore 639798 Singapore
  • Zhendong Dai
    Institute of Bio‐Inspired Structure and Surface Engineering Nanjing University of Aeronautics and Astronautics 29 Yudao Street Nanjing 210016 China
  • Keju Ji
    Institute of Bio‐Inspired Structure and Surface Engineering Nanjing University of Aeronautics and Astronautics 29 Yudao Street Nanjing 210016 China
  • Hui Jiang
    School of Materials Science and Engineering Nanyang Technological University 50 Nanyang Avenue Singapore 639798 Singapore
  • Xiaodong Chen
    School of Materials Science and Engineering Nanyang Technological University 50 Nanyang Avenue Singapore 639798 Singapore
  • Yi Long
    School of Materials Science and Engineering Nanyang Technological University 50 Nanyang Avenue Singapore 639798 Singapore

書誌事項

公開日
2018-11-14
権利情報
  • http://onlinelibrary.wiley.com/termsAndConditions#vor
DOI
  • 10.1002/adfm.201806220
公開者
Wiley

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説明

<jats:title>Abstract</jats:title><jats:p>High conductivity, large mechanical strength, and elongation are important parameters for soft electronic applications. However, it is difficult to find a material with balanced electronic and mechanical performance. Here, a simple method is developed to introduce ion‐rich pores into strong hydrogel matrix and fabricate a novel ionic conductive hydrogel with a high level of electronic and mechanical properties. The proposed ionic conductive hydrogel is achieved by physically cross‐linking the tough biocompatible polyvinyl alcohol (PVA) gel as the matrix and embedding hydroxypropyl cellulose (HPC) biopolymer fibers inside matrix followed by salt solution soaking. The wrinkle and dense structure induced by salting in PVA matrix provides large stress (1.3 MPa) and strain (975%). The well‐distributed porous structure as well as ion migration–facilitated ion‐rich environment generated by embedded HPC fibers dramatically enhances ionic conductivity (up to 3.4 S m<jats:sup>−1</jats:sup>, at <jats:italic>f</jats:italic> = 1 MHz). The conductive hybrid hydrogel can work as an artificial nerve in a 3D printed robotic hand, allowing passing of stable and tunable electrical signals and full recovery under robotic hand finger movements. This natural rubber‐like ionic conductive hydrogel has a promising application in artificial flexible electronics.</jats:p>

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