Cytochrome <i>c</i>‐Capped Fluorescent Gold Nanoclusters: Imaging of Live Cells and Delivery of Cytochrome <i>c</i>

  • Shyamtanu Chattoraj
    Department of Physical Chemistry Indian Association for the Cultivation of Science, Jadavpur Kolkata 700 032 India), Fax: (91)-33-2473-2805
  • Md. Asif Amin
    Department of Physical Chemistry Indian Association for the Cultivation of Science, Jadavpur Kolkata 700 032 India), Fax: (91)-33-2473-2805
  • Kankan Bhattacharyya
    Department of Physical Chemistry Indian Association for the Cultivation of Science, Jadavpur Kolkata 700 032 India), Fax: (91)-33-2473-2805

書誌事項

公開日
2016-04-06
権利情報
  • http://onlinelibrary.wiley.com/termsAndConditions#vor
DOI
  • 10.1002/cphc.201501163
公開者
Wiley

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説明

<jats:title>Abstract</jats:title><jats:p>Cytochrome <jats:italic>c</jats:italic>‐capped fluorescent gold nanoclusters (Au‐NCs) are used for imaging of live lung and breast cells. Delivery of cytochrome <jats:italic>c</jats:italic> inside the cells is confirmed by covalently attaching a fluorophore (Alexa Fluor 594) to cytochrome <jats:italic>c</jats:italic>‐capped Au‐NCs and observing fluorescence from Alexa 594 inside the cell. Mass spectrometry studies suggest that in bulk water, addition of glutathione (GSH) to cytochrome <jats:italic>c</jats:italic>‐capped Au‐NCs results in the formation of glutathione‐capped Au‐NCs and free apo‐cytochrome <jats:italic>c</jats:italic>. Thus glutathione displaces cytochrome <jats:italic>c</jats:italic> as a capping agent. Using confocal microscopy, the emission spectra and decay of Au‐NCs are measured in live cells. From the position of the emission maximum it is shown that the Au‐NCs exist as Au<jats:sub>8</jats:sub> in bulk water and as Au<jats:sub>13</jats:sub> inside the cells. Fluorescence resonance energy transfer from cytochrome <jats:italic>c</jats:italic>–Au‐NC (donor) to Mitotracker Orange (acceptor) indicates that the Au‐NCs localise in the mitochondria of live cells.</jats:p>

収録刊行物

  • ChemPhysChem

    ChemPhysChem 17 (13), 2088-2095, 2016-04-06

    Wiley

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