Electrolytes induce long-range orientational order and free energy changes in the H-bond network of bulk water
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- Yixing Chen
- Laboratory for fundamental BioPhotonics, Institutes of Bioengineering and Materials Science and Engineering, School of Engineering, and Lausanne Centre for Ultrafast Science, École Polytechnique Fédérale de Lausanne (EPFL), CH-1015 Lausanne, Switzerland.
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- Halil I. Okur
- Department of Chemistry, Pennsylvania State University, University Park, PA 16802, USA.
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- Nikolaos Gomopoulos
- Laboratory for fundamental BioPhotonics, Institutes of Bioengineering and Materials Science and Engineering, School of Engineering, and Lausanne Centre for Ultrafast Science, École Polytechnique Fédérale de Lausanne (EPFL), CH-1015 Lausanne, Switzerland.
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- Carlos Macias-Romero
- Laboratory for fundamental BioPhotonics, Institutes of Bioengineering and Materials Science and Engineering, School of Engineering, and Lausanne Centre for Ultrafast Science, École Polytechnique Fédérale de Lausanne (EPFL), CH-1015 Lausanne, Switzerland.
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- Paul S. Cremer
- Department of Chemistry, Pennsylvania State University, University Park, PA 16802, USA.
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- Poul B. Petersen
- Department of Chemistry and Chemical Biology, Cornell University, Ithaca, NY 14853, USA.
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- Gabriele Tocci
- Laboratory for fundamental BioPhotonics, Institutes of Bioengineering and Materials Science and Engineering, School of Engineering, and Lausanne Centre for Ultrafast Science, École Polytechnique Fédérale de Lausanne (EPFL), CH-1015 Lausanne, Switzerland.
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- David M. Wilkins
- Physical and Theoretical Chemistry Laboratory, University of Oxford, South Parks Road, Oxford OX1 3QZ, UK.
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- Chungwen Liang
- Laboratory of Computational Science and Modeling, Institute of Materials Science and Engineering, School of Engineering, École Polytechnique Fédérale de Lausanne (EPFL), CH-1015 Lausanne, Switzerland.
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- Michele Ceriotti
- Laboratory of Computational Science and Modeling, Institute of Materials Science and Engineering, School of Engineering, École Polytechnique Fédérale de Lausanne (EPFL), CH-1015 Lausanne, Switzerland.
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- Sylvie Roke
- Laboratory for fundamental BioPhotonics, Institutes of Bioengineering and Materials Science and Engineering, School of Engineering, and Lausanne Centre for Ultrafast Science, École Polytechnique Fédérale de Lausanne (EPFL), CH-1015 Lausanne, Switzerland.
書誌事項
- 公開日
- 2016-04
- DOI
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- 10.1126/sciadv.1501891
- 公開者
- American Association for the Advancement of Science (AAAS)
説明
<jats:p> Ions induce changes in the H-bond network of water that extend by >20 nm, vary for H <jats:sub>2</jats:sub> O and D <jats:sub>2</jats:sub> O, and lead to surface tension anomalies. </jats:p>
収録刊行物
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- Science Advances
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Science Advances 2 (4), e1501891-, 2016-04
American Association for the Advancement of Science (AAAS)