A Stable Single Piece of Unimolecularly π-Stacked Porphyrin Aggregate in a Thixotropic Low Molecular Weight Gel:  A One-Dimensional Molecular Template for Polydiacetylene Wiring up to Several Tens of Micrometers in Length

  • Michihiro Shirakawa
    Department of Chemistry & Biochemistry, Graduate School of Engineering, Kyushu University, Fukuoka 812-8581, Japan
  • Norifumi Fujita
    Department of Chemistry & Biochemistry, Graduate School of Engineering, Kyushu University, Fukuoka 812-8581, Japan
  • Seiji Shinkai
    Department of Chemistry & Biochemistry, Graduate School of Engineering, Kyushu University, Fukuoka 812-8581, Japan

書誌事項

公開日
2005-03-01
DOI
  • 10.1021/ja042869d
公開者
American Chemical Society (ACS)

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説明

An amide-type copper porphyrin gelator having alkyldiacetylene tethers gives very transparent gel in Decalin, and the gel shows unique thixotropic behavior. One-dimensional aggregates generated in the gel act as templates for unimolecularly segregated polydiacetylene wiring upon UV irradiation on the surface. The polymerization along the aggregation goes to at least several micrometers long.

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