Role of metal–molecule chemistry and interdiffusion on the electrical properties of an organic interface: The Al–F16CuPc case

  • Chongfei Shen
    Department of Electrical Engineering and Princeton Materials Institute, Princeton University, Princeton, New Jersey 08544
  • Antoine Kahn
    Department of Electrical Engineering and Princeton Materials Institute, Princeton University, Princeton, New Jersey 08544
  • Jeffrey Schwartz
    Department of Chemistry, Princeton University, Princeton, New Jersey 08544

書誌事項

公開日
2001-12-15
DOI
  • 10.1063/1.1419263
公開者
AIP Publishing

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説明

<jats:p>The chemistry and electronic structure of interfaces between Al and copper hexadecafluorophthalocyanine (F16CuPc) are studied via x-ray photoemission spectroscopy, ultraviolet photoemission spectroscopy (UPS), and current–voltage measurements. Electron injection barriers measured by UPS are reported. Analysis of the Al–F16CuPc reaction shows the formation of a phase of three-dimensional (F16CuPc)3Al species. The reacted region is extended at the Al-on-F16CuPc interface and narrow at the F16CuPc-on-Al interface. A series of metal/F16CuPc/metal structures is fabricated to study the impact of the interface chemistry and deposition sequence on device performances. It is found that (F16CuPc)3Al forms a low conductivity region, which has considerable bearing on the electron current. The interface fabrication sequence, which defines the thickness of the reacted region, therefore has a profound impact on device performance.</jats:p>

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