The hydrogenolysis of diarylmethane

書誌事項

公開日
1988-10
権利情報
  • https://www.elsevier.com/tdm/userlicense/1.0/
DOI
  • 10.1016/0016-2361(88)90137-8
公開者
Elsevier BV

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説明

Abstract The thermal decomposition of the diarylmethane in hydrogen-donor solvents proceeds via the ipso-addition of a hydrogen atom transferred from the solvent. This reaction is slow in tetralin at temperatures of 430–460 °C, but it is promoted by a binary solvent system composed of tetralin and dibenzyl (20:1 molar ratio), and its ability to donate hydrogen is comparable with that of 9,10-dihydroanthracene. The additive effect of 1H-phenalene as a source of phenalenyl radical is half that of dibenzyl. The addition of a hydrogen shuttler such as anthracene and phenanthrene to tetralin also promotes the above reaction, but their additive effect is modest, compared with the hydrogen-donating abilities of the corresponding dihydro-derivatives.

収録刊行物

  • Fuel

    Fuel 67 (10), 1436-1440, 1988-10

    Elsevier BV

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