Formation of a Pt<sub>12</sub> Cluster by Single‐Atom Control That Leads to Enhanced Reactivity: Hydrogenation of Unreactive Olefins

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書誌事項

公開日
2013-05-31
権利情報
  • http://onlinelibrary.wiley.com/termsAndConditions#vor
DOI
  • 10.1002/ange.201302860
  • 10.1002/anie.201302860
公開者
Wiley

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説明

A platinum subnanocluster catalyst composed of 12 atoms was synthesized using a phenylazomethine dendrimer, which can assemble twelve PtCl4 units by stepwise complexation, followed by reduction to Pt(0). Unreactive olefins that were not activated by conventional 2 nm Pt nanoparticles were successfully hydrogenated by the subnanocluster. EWG = electron-withdrawing group.

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