Crystal structure of corundum type Mg4(Nb2–xTax)O9 microwave dielectric ceramics with low dielectric loss

書誌事項

公開日
2003-01
権利情報
  • https://www.elsevier.com/tdm/userlicense/1.0/
DOI
  • 10.1016/s0955-2219(03)00167-5
公開者
Elsevier BV

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説明

Abstract New microwave dielectric ceramics, i.e. Mg 4 (Nb 2− x Ta x )O 9 (MNT) solid solutions, were synthesized and their microwave dielectric properties and crystal structure were investigated in this study. From the discrete variational Xα (DV-Xα) method, it was found that the Ta–O bonds in the TaO 6 octahedron become more covalent than Nb–O bonds in the NbO 6 octahedron; this result leads to the decrease of the ionicity in the Ta 5+ ion. The dielectric constants of MNT were slightly decreased from 12.4 to 11.5; this result might be due to the covalent interaction of Ta–O bonding. The quality factors of the samples were found to exhibit high value ( Q · f ≒350 000 GHz for x =2) which is comparable to those of Al 2 O 3 .

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