Elasticity of (Mg,Fe)O Through the Spin Transition of Iron in the Lower Mantle

  • J. C. Crowhurst
    Chemistry, Materials, and Life Sciences Directorate, Lawrence Livermore National Laboratory (LLNL), Livermore, CA 94550, USA.
  • J. M. Brown
    Chemistry, Materials, and Life Sciences Directorate, Lawrence Livermore National Laboratory (LLNL), Livermore, CA 94550, USA.
  • A. F. Goncharov
    Chemistry, Materials, and Life Sciences Directorate, Lawrence Livermore National Laboratory (LLNL), Livermore, CA 94550, USA.
  • S. D. Jacobsen
    Chemistry, Materials, and Life Sciences Directorate, Lawrence Livermore National Laboratory (LLNL), Livermore, CA 94550, USA.

書誌事項

公開日
2008-01-25
DOI
  • 10.1126/science.1149606
公開者
American Association for the Advancement of Science (AAAS)

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説明

<jats:p> Changes in the electronic configuration of iron at high pressures toward a spin-paired state within host minerals ferropericlase and silicate perovskite may directly influence the seismic velocity structure of Earth's lower mantle. We measured the complete elastic tensor of ferropericlase, (Mg <jats:sub> 1– <jats:italic>x</jats:italic> </jats:sub> ,Fe <jats:sub> <jats:italic>x</jats:italic> </jats:sub> )O ( <jats:italic>x</jats:italic> = 0.06), through the spin transition of iron, whereupon the elastic moduli exhibited up to 25% softening over an extended pressure range from 40 to 60 gigapascals. These results are fully consistent with a simple thermodynamic description of the transition. Examination of previous compression data shows that the magnitude of softening increases with iron content up to at least <jats:italic>x</jats:italic> = 0.20. Although the spin transition in (Mg,Fe)O is too broad to produce an abrupt seismic discontinuity in the lower mantle, the transition will produce a correlated negative anomaly for both compressional and shear velocities that extends throughout most, if not all, of the lower mantle. </jats:p>

収録刊行物

  • Science

    Science 319 (5862), 451-453, 2008-01-25

    American Association for the Advancement of Science (AAAS)

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