High-Field Magnetization and Neutron Diffraction Studies of One-Dimensional Compound Ca<sub>3</sub>CoRhO<sub>6</sub>

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  • Niitaka Seiji
    Department of Chemistry, Graduate School of Science, Kyoto University, Kyoto 606-8502
  • Kageyama Hiroshi
    Institute for Solid State Physics, University of Tokyo, Kashiwanoha, Kashiwa, Chiba 277-8581
  • Yoshimura Kazuyoshi
    Department of Chemistry, Graduate School of Science, Kyoto University, Kyoto 606-8502
  • Kosuge Koji
    Department of Chemistry, Graduate School of Science, Kyoto University, Kyoto 606-8502
  • Kawano Shinji
    Research Reactor Institute, Kyoto University, Kumatori, Sennan, Osaka 590-0494
  • Aso Naofumi
    Neutron Scattering Laboratory, Institute for Solid State Physics, University of Tokyo, Shirakata 106-1, Tokai-mura, Ibaraki 319-1106
  • Mitsuda Akihiro
    Institute for Solid State Physics, University of Tokyo, Kashiwanoha, Kashiwa, Chiba 277-8581
  • Mitamura Hiroyuki
    Institute for Solid State Physics, University of Tokyo, Kashiwanoha, Kashiwa, Chiba 277-8581
  • Goto Tsuneaki
    Institute for Solid State Physics, University of Tokyo, Kashiwanoha, Kashiwa, Chiba 277-8581

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  • High-Field Magnetization and Neutron Diffraction Studies of One-Dimensional Compound Ca3CoRhO6.

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High-field magnetization and neutron diffraction measurements were performed on the one-dimensional compound Ca3CoRhO6. The long-range ordered state was first observed below 90 K. A plateau at 1/3 of the saturation magnetization was observed in the magnetization curve at 70 K, indicating ferrimagnetic alignment of the ferromagnetic Ising chains. We also observed a large hysteresis originating from a spin freezing of ferromagnetic chains in the magnetization curve at 4.2 K. Based on the results of high-field magnetization and neutron diffraction measurements, a possible magnetic structure is discussed in terms of the spin frustration on the triangular lattice.

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