Theory of Viscoelasticity in Temporarily Crosslinked Polymers (III)

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  • Hayashi Shizuo
    Department of Physics, Faculty of Liberal Arts and Education, Gunma University

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Viscoelasticity of network structure is investigated using the Rouse model corresponding to macro-Brownian motion. The viscous and elastic effects between chains are introduced and a slip equation determining the slip rate of chain and the stress are obtained in a clearer form than in the preceding report. Stress relaxation, stationary simple elongation, stationary flow and periodic shear deformation are treated. The relaxation spectrum given by the theory is of the box type and the viscosity coefficient and the time rate of energy dissipation are proportional to the 3.4th power of molecular weight.

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