Development of High-Pressure High-Temperature NMR Probe and Dynamics, Structure and Reactions in Supercritical Water

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  • YOSHIDA Ken
    Department of Chemical Science and Technology, Faculty of Engineering, University of Tokushima

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  • 高圧高温NMR分光法の開発と超臨界水中のダイナミクス・構造・反応の研究
  • 受賞記念解説 : 高圧力学会奨励賞 高圧高温NMR分光法の開発と超臨界水中のダイナミクス・構造・反応の研究
  • ジュショウ キネン カイセツ : コウアツリョク ガッカイ ショウレイショウ コウアツ コウオン NMR ブンコウホウ ノ カイハツ ト チョウリンカイ スイチュウ ノ ダイナミクス ・ コウゾウ ・ ハンノウ ノ ケンキュウ

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  The present review introduces our recent studies of the title subjects that have led to the JSHPST Award for Young Scientists, 2011. We studied the structure, dynamics, and reactions in water under high-pressure and high-temperature conditions using NMR and computational methods. The NMR apparatus was newly developed and was applied for the self-diffusion measurements of water and nonpolar organic fluids over a wide range of pressure and temperature. Molecular dynamics simulation combined with a new analysis scheme provided new insights into the translational dynamics in the supercritical water in the medium-density region in relation to the structure and lifetime of the solvation shell.<br>

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