Impacts of Additional HONO Sources on Concentrations and Deposition of NO<sub>y</sub> in the Beijing-Tianjin-Hebei Region of China

  • Li Ying
    State Key Laboratory of Atmospheric Boundary Layer Physics and Atmospheric Chemistry (LAPC), Institute of Atmospheric Physics, Chinese Academy of Sciences
  • An Junling
    State Key Laboratory of Atmospheric Boundary Layer Physics and Atmospheric Chemistry (LAPC), Institute of Atmospheric Physics, Chinese Academy of Sciences
  • Kajino Mizuo
    Meteorological Research Institute
  • Li Jian
    State Key Laboratory of Atmospheric Boundary Layer Physics and Atmospheric Chemistry (LAPC), Institute of Atmospheric Physics, Chinese Academy of Sciences
  • Qu Yu
    State Key Laboratory of Atmospheric Boundary Layer Physics and Atmospheric Chemistry (LAPC), Institute of Atmospheric Physics, Chinese Academy of Sciences

書誌事項

公開日
2015
DOI
  • 10.2151/sola.2015-009
公開者
公益社団法人 日本気象学会

説明

This study applies the chemistry version of the Weather Research and Forecasting model (WRF-Chem) to examine impacts of three additional HONO sources, i.e., the reaction of photo-excited NO2 (NO2*) with water vapor (NO2* chemistry), the NO2 heterogeneous reaction on aerosol surfaces and HONO emissions, on concentrations and deposition of individual NOy species over the Beijing-Tianjin-Hebei region (BTH) in summer and winter periods of 2007. The results show that the three additional HONO sources produce a 20%∼40% (> 100%) increase in monthly-mean OH concentrations in many urban areas in August (February), leading to a 10%∼40% (10%∼100%) variation in monthly-mean concentrations of NOx, NO3 and PAN, a 5%∼10% (10%∼40%) increase in the total dry deposition of NOy, and an enhancement of 1.4 Gg N (1.5 Gg N) in the total of dry and wet deposition of NOy over this region in August (February). These results suggest that the additional HONO sources aggravate regional-scale acid deposition, emphasizing the importance of the additional HONO sources in the NOy budget.

収録刊行物

  • SOLA

    SOLA 11 (0), 36-42, 2015

    公益社団法人 日本気象学会

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