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Development of Model-free Analysis Method on Quasi-elastic Neutron Scattering and Application to Liquid Water
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- Kikuchi Tatsuya
- J-PARC Center, Japan Atomic Energy Agency
Bibliographic Information
- Other Title
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- 中性子準弾性散乱に向けたモデルフリー解析法の開発とその水への応用
- 受賞記事 中性子準弾性散乱に向けたモデルフリー解析法の開発とその水への応用
- ジュショウ キジ チュウセイシ ジュンダンセイ サンラン ニ ムケタ モデルフリー カイセキホウ ノ カイハツ ト ソノ ミズ エ ノ オウヨウ
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Description
<p>In general, analysis of quasi-elastic neutron scattering spectra needs some mathematical models in its process, and hence the obtained result is a model dependent. Model-dependent analysis may lead misunderstandings caused by inappropriate initial models or may miss an unexpected relaxation phenomenon. We have developed an analysis method for processing QENS data without a specific model, which we call as mode-distribution analysis. In this method, we supposed that all modes can be described as combinations of the relaxations based on the exponential law. By this method, we can obtain a distribution function B (Q, Γ) which we call the mode-distribution function, to represent the number of relaxation modes and distributions of the relaxation times in the modes. We report the first application to experimental data of liquid water. In addition to the two known modes, the existence of a relaxation mode of water molecules with an intermediate time scale has been discovered.</p>
Journal
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- hamon
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hamon 24 (2), 106-110, 2014
The Japanese Society for Neutron Science
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Keywords
Details 詳細情報について
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- CRID
- 1390001288094267776
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- NII Article ID
- 130007510520
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- NII Book ID
- AA11905115
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- ISSN
- 1884636X
- 1349046X
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- NDL BIB ID
- 025521299
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- Text Lang
- ja
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- Data Source
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- JaLC
- NDL Search
- Crossref
- CiNii Articles
- OpenAIRE
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- Abstract License Flag
- Disallowed