New Development of Photo-induced Electron Transfer Events in Non-covalently Assemblies

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  • SUGA Yasuhiro
    National Institute of Materials and Chemical Research, COE laboratory
  • ARIMURA Takashi
    National Institute of Materials and Chemical Research, COE laboratory

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  • 非共有結合型光誘超電子移動研究の新展開
  • ヒキョウユウ ケツゴウガタ ヒカリ ユウキ デンシ イドウ ケンキュウ ノ シン テンカイ

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Abstract

Electron-transfer (ET) reactions in metalloproteins play an important role in both photosynthesis and respiratory oxidative phosphorylation. In spite of this importance, the exact nature of specific partner-to-partner in ET processes is still poorly understood. In terms of specifics, a lot of chemists have tested the importance of three different kinds of non-covalent pathway interactions that are proposed to play a critical role in mediating biological ET events, namely : (1) van der Waals associations, (2) Electrostatic contacts, (3) Hydrogen bonds. This review summarizes the recent development of new, non-covalently approaches to ET modeling.

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