Construction of Optically Active Isotwistanes and Aminocyclitols Using Chiral Cyclohexadiene as a Common Intermediate

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  • Harada Shinji
    Graduate School of Pharmaceutical Sciences, Chiba University Molecular Chirality Research Center, Chiba University
  • Li Kexin
    Graduate School of Pharmaceutical Sciences, Chiba University
  • Kino Ryuto
    Graduate School of Pharmaceutical Sciences, Chiba University
  • Takeda Takuya
    Graduate School of Pharmaceutical Sciences, Chiba University
  • Wu Chia-Hsien
    Graduate School of Pharmaceutical Sciences, Chiba University Department of Chemistry, National Tsing Hua University
  • Hiraoka Shiharu
    Graduate School of Pharmaceutical Sciences, Chiba University
  • Nishida Atsushi
    Graduate School of Pharmaceutical Sciences, Chiba University Molecular Chirality Research Center, Chiba University

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<p>We have developed a new method for synthesizing chiral isotwistane and homoisotwistane skeletons as well as aminocyclitols in a highly stereoselective manner. These results were achieved through the use of a common intermediate, which was derived from the ytterbium-catalyzed asymmetric Diels–Alder reaction of Danishefsky diene.</p>

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