Evaluation and Application of Liquid Chromatographic Columns Coated with "Intelligent" Ligands(3)Immobilized Enzyme Phospholipid Column
-
- KAMIMORI Hiroshi
- Shionogi Research Laboratories, Shionogi & Co., Ltd.
-
- KONISHI Masaharu
- Shionogi Research Laboratories, Shionogi & Co., Ltd.
書誌事項
- タイトル別名
-
- Evaluation and Application of Liquid Chromatographic Columns Coated with "Intelligent" Ligands. (III). Immobilized Enzyme Phospholipid Column.
この論文をさがす
説明
Immobilized enzyme columns have been developed for use as high-performance liquid chromatographic enzyme reactors. Enzyme reactors were prepared by immobilizing trypsin or cytochrome-c on phospholipid columns. Dynamic coating was employed to prepare the reactors by recycling a buffer solution containing trypsin or cytochrome-c through a phospholipid-coated column, on which the enzymes were immobilized by hydrophobic binding. The immobilized trypsin column displayed hydrolytic activity which catalyzed the hydrolysis of L-amino acid esters to amino acid. The immobilized cytochrome-c column exhibited oxidation activity which catalyzed N-demethylation of N,N-dimethylaniline, codeine, and dihydrocodeine in the presence of hydrogen peroxide as an oxygenating agent. The enzyme reaction proceeded rapidly in the column; both product and substrate could be separated and detected simultaneously. The immobilized enzyme columns could be readily regenerated using the original phospholipid column by repeating the dynamic coating. These immobilized enzyme columns could be utilized as enzyme reactors in the high-performance liquid chromatographic mode. Complete hydrolysis of amino acid ester was observed with the trypsin column. Demethylation of codeine and of dihydrocodeine were observed with the cytchrome-c column.
収録刊行物
-
- Analytical Sciences
-
Analytical Sciences 17 (9), 1085-1089, 2001
社団法人 日本分析化学会
- Tweet
キーワード
詳細情報 詳細情報について
-
- CRID
- 1390282679234049536
-
- NII論文ID
- 10007177835
-
- NII書誌ID
- AA10500785
-
- COI
- 1:CAS:528:DC%2BD3MXntFWquro%3D
-
- ISSN
- 13482246
- 09106340
-
- NDL書誌ID
- 5912278
-
- PubMed
- 11708064
-
- 本文言語コード
- en
-
- 資料種別
- journal article
-
- データソース種別
-
- JaLC
- NDLサーチ
- Crossref
- PubMed
- CiNii Articles
-
- 抄録ライセンスフラグ
- 使用不可