Broadband Vibrational Sum Frequency Generation Spectroscopy of a Liquid Surface.
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- HOMMEL Elizabeth L.
- The Ohio State University, Department of Chemistry
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- MA Gang
- The Ohio State University, Department of Chemistry
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- ALLE Heather C.
- The Ohio State University, Department of Chemistry
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Abstract
An important advance in surface science has been the evolution of sum frequency generation to the application of studying surface structure and chemistry of liquid surfaces at the molecular-level by probing the vibrational signatures of surface molecules. Recently, broad-bandwidth sum frequency generation (BBSFG) spectroscopy has become an important tool for investigating gas-solid interfaces. BBSFG spectroscopy allows, theoretically, a surface sum frequency spectrum to be acquired within one pulse of the laser. In this paper, the viability of BBSFG to study inherently small nonlinear response interfaces and the time-resolving capability of this surface-selective technology are demonstrated. Presented here are the first published accounts of spectra from a liquid surface utilizing the broad-bandwidth sum frequency technology with acquisition times as low as 500 milliseconds.
Journal
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- Analytical Sciences
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Analytical Sciences 17 (11), 1325-1329, 2001
The Japan Society for Analytical Chemistry
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Keywords
Details 詳細情報について
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- CRID
- 1390282679234866944
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- NII Article ID
- 130004440344
- 10007419514
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- NII Book ID
- AA10500785
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- COI
- 1:CAS:528:DC%2BD3MXos1Ogs7o%3D
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- ISSN
- 13482246
- 09106340
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- NDL BIB ID
- 5982317
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- PubMed
- 11759518
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- Text Lang
- en
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- Data Source
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- JaLC
- NDL
- Crossref
- PubMed
- CiNii Articles
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- Abstract License Flag
- Disallowed