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Construcution of a Complete Bioelectrocatalytic Electrode Composed of Alcohol Dehydrogenase- and All Electron-transfer Components-modified Graphite Felt for Diol Oxidation
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- Kashiwagi Yoshitomo
- Faculty of Pharmaceutical Sciences, Tohoku University
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- Pan Qinghai
- Faculty of Pharmaceutical Sciences, Tohoku University
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- Kurashima Futoshi
- Faculty of Pharmaceutical Sciences, Tohoku University
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- Kikuchi Chikara
- Faculty of Pharmaceutical Sciences, Tohoku University
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- Anzai Jun-ichi
- Faculty of Pharmaceutical Sciences, Tohoku University
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- Osa Tetsuo
- Faculty of Pharmaceutical Sciences, Tohoku University
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Description
A poly(acrylic acid)-coated graphite felt electrode immobilizing all bioelectrochemical reaction components of ferrocene, diaphorase, NADH and alcohol dehydrogenase in the domain of the poly(acrylic acid) layer was applied to oxidize electrocatalytically cis-1,2-cyclohexanedimethanol and 3-methyl-1,5-pentanediol to (+)-(1R, 6S)-cis-8-oxabicyclo[4.3.0]nonan-7-one and (3S)-3-methyl-δ-valerolactone, respectively, in a 0.15 M phosphate buffer (pH 8.0) at the constant potential of 0.45 V vs. SCE with high current efficiency (>92%) and high optical purity (>92%).
Journal
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- Chemistry Letters
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Chemistry Letters 27 (2), 143-144, 1998
The Chemical Society of Japan
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Keywords
Details 詳細情報について
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- CRID
- 1390282679552761600
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- NII Article ID
- 130004420907
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- COI
- 1:CAS:528:DyaK1cXhtFWlu7Y%3D
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- ISSN
- 13480715
- 03667022
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- Text Lang
- en
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- Data Source
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- JaLC
- Crossref
- CiNii Articles
- OpenAIRE
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- Abstract License Flag
- Disallowed