A Demonstration Test to Separate Minor Actinides in High-Level Liquid Waste by <i>N,N,N',N',N'',N''</i>-Hexaoctyl Nitrilotriacetamide (HONTA) Using Mixer-Settler Extractors in a Hot Cell
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- BAN Yasutoshi
- Research Group for Nuclear Fuel Cycle Science, Nuclear Science and Engineering Center, Japan Atomic Energy Agency
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- SUZUKI Hideya
- Research Group for Nuclear Fuel Cycle Science, Nuclear Science and Engineering Center, Japan Atomic Energy Agency
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- HOTOKU Shinobu
- Research Group for Nuclear Fuel Cycle Science, Nuclear Science and Engineering Center, Japan Atomic Energy Agency
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- TSUBATA Yasuhiro
- Research Group for Nuclear Fuel Cycle Science, Nuclear Science and Engineering Center, Japan Atomic Energy Agency
抄録
<p>A demonstration test was performed to separate minor actinides (MA; Am and Cm) by N,N,N',N',N'',N''-hexaoctyl nitrilotriacetamide (HONTA) as an extractant using mixer-settler extractors installed in a hot cell. A high-level liquid waste containing MA, and rare earths (RE; Y, La, Nd, and Eu) was used as the feed. HONTA diluted to 0.05 mol/dm3 in n-dodecane was fed as the organic phase, and a part of the organic phase was reused without solvent regeneration. HONTA effectively extracted MA, whereas RE were less extractable. Consequently, the Y, La, Nd, and Eu ratios distributed to a RE fraction were >99.9%, 99.2%, 61.8%, and 81.4%, respectively. The Am and Cm ratios distributed to an MA fraction were 86.8% and 74.7%, respectively, and a substantial amount of MA (0.12 g) was recovered in the MA fraction by the end of the cumulative duration of 40 h. </p>
収録刊行物
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- Solvent Extraction Research and Development, Japan
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Solvent Extraction Research and Development, Japan 31 (1), 1-11, 2024
日本溶媒抽出学会
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詳細情報 詳細情報について
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- CRID
- 1390581025652071040
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- ISSN
- 21884765
- 13417215
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- 本文言語コード
- en
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- データソース種別
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- JaLC
- Crossref
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- 抄録ライセンスフラグ
- 使用不可