Photophysics and photochemical dynamics of chlorotoluene molecule

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Abstract Laser-induced fluorescence spectra of jet-cooled chlorotoluene molecules are reported for the S 1 state. The fluorescence excitation spectrum of m -chlorotoluene shows some low-frequency bands up to 200 cm −1 above the S 1 origin, which are assigned to internal rotational modes of the methyl group. Beyond 300 cm −1 and up to approximately 1500 cm −1 sharp vibrational bands are observed, which are assigned by measurement of the dispersed fluorescence spectrum on excitation of each vibrational band. The vibrational energies of the CCl stretching modes for the o- , m - and p -chlorotoluene molecules are 341, 378 and 360 cm −1 respectively in the S 1 state.

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