The Synthesis and Property of Dihydropyrene Derivatives Containing a Nitrogen Atom

書誌事項

公開日
2007-08-10
DOI
  • 10.1080/15421400701503667
公開者
Informa UK Limited

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説明

Dihydropyrene (DHP) is 14π aromatic compound and applied as an aromatic probe by chemical shift of internal methyl groups in 1H-NMR spectra. DHP containing a nitrogen atom 1a and 2a were designed as photochromic compounds which were restrained thermal-isomerization. 1a and 2a were confirmed as DHP types by 1H-NMR spectra. Chemical shifts of internal methyl groups of 1a and 2a were observed at the lower magnetic field than that of DHP 3a . According to optimized structures of 1a and 3a , it was expected that the internal methyl group located of the out at center of 14π annulene ring. Isomerization to [2.2]metacyclophanediene 1b from DHP 1a by photo-irradiation of visible light was not observed.

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