Korringa-like relaxation in the high-temperature phase of<mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline"><mml:mi>A</mml:mi></mml:math>-site ordered YBaMn<mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline"><mml:msub><mml:mrow /><mml:mn>2</mml:mn></mml:msub></mml:math>O<mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline"><mml:msub><mml:mrow /><mml:mn>6</mml:mn></mml:msub></mml:math>
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説明
We report on high-temperature electron spin resonance studies of A-site ordered YBaMn2O6 and disordered Y0.5Ba0.5MnO3. In the disordered sample we find that the linewidth is governed by spin-spin relaxation processes as in many other manganite systems. In contrast we find a Korringa-like spin relaxation with a slope of about 1 Oe/K above the charge-ordering transition and extending up to 930K in the metal ordered YBaMn2O6 samples. A Korringa-law is a clear feature of a truly metallic state, pointing to an unconventional high-temperature phase of these ordered manganites. In agreement with the ESR intensity this suggests that in the metallic high-temperature phase the ESR signal stems from Mn^4+ core spins which relax via the quasi-delocalized e_g electrons.
収録刊行物
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- Physical Review B
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Physical Review B 85 2012-05-11
American Physical Society (APS)
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詳細情報 詳細情報について
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- CRID
- 1873398392284123904
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- ISSN
- 1550235X
- 10980121
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- データソース種別
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- OpenAIRE