Photocatalytic C−C Bond Cleavage and Amination of Cycloalkanols by Cerium(III) Chloride Complex

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  • Jing‐Jing Guo
    School of Physical Science and Technology ShanghaiTech University Shanghai 201210 China
  • Anhua Hu
    School of Physical Science and Technology ShanghaiTech University Shanghai 201210 China
  • Yilin Chen
    School of Physical Science and Technology ShanghaiTech University Shanghai 201210 China
  • Jianfeng Sun
    School of Physical Science and Technology ShanghaiTech University Shanghai 201210 China
  • Haoming Tang
    School of Physical Science and Technology ShanghaiTech University Shanghai 201210 China
  • Zhiwei Zuo
    School of Physical Science and Technology ShanghaiTech University Shanghai 201210 China

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Published
2016-11-11
Rights Information
  • http://onlinelibrary.wiley.com/termsAndConditions#vor
DOI
  • 10.1002/ange.201609035
Publisher
Wiley

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<jats:title>Abstract</jats:title><jats:p>A general strategy for the cleavage and amination of C−C bonds of cycloalkanols has been achieved through visible‐light‐induced photoredox catalysis utilizing a cerium(III) chloride complex. This operationally simple methodology has been successfully applied to a wide array of unstrained cyclic alcohols, and represents the first example of catalytic C−C bond cleavage and functionalization of unstrained secondary cycloalkanols.</jats:p>

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