Facile Synthesis of Highly π-Extended Heteroarenes, Dinaphtho[2,3-<i>b</i>:2‘,3‘-<i>f</i>]chalcogenopheno[3,2-<i>b</i>]chalcogenophenes, and Their Application to Field-Effect Transistors

  • Tatsuya Yamamoto
    Department of Applied Chemistry, Graduate School of Engineering, Hiroshima University, Higashi-Hiroshima 739-8527, Japan, and Institute for Advanced Materials Research, Hiroshima University, Higashi-Hiroshima 739-8530, Japan
  • Kazuo Takimiya
    Department of Applied Chemistry, Graduate School of Engineering, Hiroshima University, Higashi-Hiroshima 739-8527, Japan, and Institute for Advanced Materials Research, Hiroshima University, Higashi-Hiroshima 739-8530, Japan

書誌事項

公開日
2007-02-01
DOI
  • 10.1021/ja068429z
公開者
American Chemical Society (ACS)

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説明

A facile three-step synthetic procedure for highly π-extended heteroarenes, dinaphtho[2,3-b:2‘,3‘-f]thieno[3,2-b]thiophene (DNTT) and dinaphtho[2,3-b:2‘,3‘-f]selenopheno[3,2-b]selenophene (DNSS), was established. Solution UV−vis spectra and electrochemistry indicated that they have relatively low-lying HOMO levels and large HOMO−LUMO energy gaps. OFET devices fabricated with evaporated thin-films of DNTT and DNSS showed excellent FET characteristics in air, and the highest field-effect mobility of DNTT- and DNSS-based OFETs is 2.9 and 1.9 cm2 V-1 s-1, respectively.

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